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Spectral Emission Dependence of Tin‐Vacancy Centers in Diamond from Thermal Processing and Chemical Functionalization

descriptionPublicationkeyboard_double_arrow_right Article , Preprint , Other literature type 05 Nov 2021Embargo end date: 01 Jun 2021 Italy English Publisher:WileyJournal:Advanced Photonics Research, volume 3 (issn: 2699-9293, eissn: 2699-9293, Copyright policy )Funded by:MIUR | unidentified, EC | LasIonDef, EC | ASTERIQS
Authors: Corte, Emilio; Sachero, Selene; Ditalia Tchernij, Sviatoslav; Lühmann, Tobias; Pezzagna, Sébastien; Traina, Paolo; Degiovanni, Ivo Pietro; +5 Authors

doi: 10.1002/adpr.202100148 , 10.48550/arxiv.2106.07365

arXiv: 2106.07365

handle: 11696/72916 , 2318/1816585

Spectral Emission Dependence of Tin‐Vacancy Centers in Diamond from Thermal Processing and Chemical Functionalization

Abstract

A systematic photoluminescence (PL) investigation of the spectral emission properties of individual optical defects fabricated in diamond upon ion implantation and annealing is reported. Three spectral lines at 620, 631, and 647 nm are identified and attributed to the SnV center due to their occurrence in the PL spectra of the very same single‐photon emitting defects. It is shown that the relative occurrence of the three spectral features can be modified by oxidizing the sample surface following thermal annealing. The relevant emission properties of each class of individual emitters, including the excited state emission lifetime and the emission intensity saturation parameters are reported.

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Keywords

single-photon source, Quantum Physics, Condensed Matter - Materials Science, diamond, single-photon sources, charge state, ion implantation, quantum optics, materials processing, Materials Science (cond-mat.mtrl-sci), FOS: Physical sciences, QC350-467, Optics. Light, TA1501-1820, quantum, charge, diamond, annealing, ion implantation, Applied optics. Photonics, Quantum Physics (quant-ph)

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    		 15
    popularity
    This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
    		 Top 10%
    influence
    This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
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    impulse
    This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
15
Top 10%
Average
Top 10%
Green
gold