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Polarized-neutron investigation of magnetic ordering and spin dynamics in BaCo 2 (AsO 4 ) 2 frustrated honeycomb-lattice magnet

Authors: Regnault, Louis-Pierre; Boullier, Cyrille; Lorenzo, J.E.;

Polarized-neutron investigation of magnetic ordering and spin dynamics in BaCo 2 (AsO 4 ) 2 frustrated honeycomb-lattice magnet

Abstract

The magnetic properties of the cobaltite {\BCAO}, a good realization of the quasi two-dimensional frustrated honeycomb-lattice system with strong planar anisotropy, have been reinvestigated by means of spherical neutron polarimetry with CRYOPAD. From accurate measurements of polarization matrices both on elastic and inelastic contributions as a function of the scattering vector {\bf{Q}}, we have been able to determine the low-temperature magnetic structure of {\BCAO} and reveal its puzzling in-plane spin dynamics. Surprisingly, the ground-state structure (described by an incommensurate propagation vector ${\bf{k}}_{1}=(k_{x}, 0, k_{z}$), with $k_{x}=0.270{\pm}0.005$ and $k_{z} \approx -1.31$) appears to be a quasi-collinear structure, and not a simple helix, as previously determined. In addition, our results have revealed the existence of a non-negligible out-of-plane moment component $ \approx 0.25��_{B}$/Co$^{2+}$, representing about 10\% of the in-plane component, as demonstrated by the presence of finite off-diagonal elements $P_{yz}$ and $P_{zy}$ of the polarization matrix, both on elastic and inelastic magnetic contributions. Despite a clear evidence of the existence of a slightly inelastic contribution of structural origin superimposed to the magnetic excitations at the scattering vectors ${\bf{Q}}=(0.27, 0, 3.1)$ and ${\bf{Q}}=(0.73, 0, 0.8)$ (energy transfer $��E \approx 2.3$ meV), no strong inelastic nuclear-magnetic interference terms could be detected so far, meaning that the nuclear and magnetic degrees of freedom have very weak cross-correlations. The strong inelastic $P_{yz}$ and $P_{zy}$ matrix elements can be understood by assuming that the magnetic excitations in {\BCAO} are spin waves associated with trivial anisotropic precessions of the magnetic moments involved in the canted incommensurate structure.

43 pages, 16 figures

Country
France
Keywords

H1-99, Condensed Matter - Materials Science, Science (General), Strongly Correlated Electrons (cond-mat.str-el), Materials Science, Materials Science (cond-mat.mtrl-sci), FOS: Physical sciences, Condensed Matter Physics, 530, [PHYS.COND.CM-MS] Physics [physics]/Condensed Matter [cond-mat]/Materials Science [cond-mat.mtrl-sci], Article, Social sciences (General), Q1-390, Condensed Matter - Strongly Correlated Electrons, [PHYS.QPHY]Physics [physics]/Quantum Physics [quant-ph], [PHYS.COND.CM-MS]Physics [physics]/Condensed Matter [cond-mat]/Materials Science [cond-mat.mtrl-sci], [PHYS.QPHY] Physics [physics]/Quantum Physics [quant-ph]

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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
39
Top 10%
Top 10%
Top 10%
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