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Local field enhancement and thermoplasmonics in multimodal aluminum structures

Authors: Wiecha, Peter; Mennemanteuil, Marie-Maxime; Khlopin, Dmitry; Martin, Jérôme; Arbouet, Arnaud; Gérard, Davy; Bouhelier, Alexandre; +2 Authors

Local field enhancement and thermoplasmonics in multimodal aluminum structures

Abstract

Aluminum nanostructures have recently been at the focus of numerous studies due to their properties including oxidation stability and surface plasmon resonances covering the ultraviolet and visible spectral windows. In this article, we reveal a new facet of this metal relevant for both plasmonics purpose and photo-thermal conversion. The field distribution of high order plasmonic resonances existing in two-dimensional Al structures is studied by nonlinear photoluminescence (nPL) microscopy in a spectral region where electronic interband transitions occur. The polarization sensitivity of the field intensity maps shows that the electric field concentration can be addressed and controlled on-demand. We use a numerical tool based on the Green dyadic method to analyze our results and to simulate the absorbed energy that is locally converted into heat. The polarization-dependent temperature increase of the Al structures is experimentally quantitatively measured, and is in an excellent agreement with theoretical predictions. Our work highlights Al as a promising candidate for designing thermal nanosources integrated in coplanar geometries for thermally assisted nanomanipulation or biophysical applications.

8 pages 6 figures main article; 7 pages 9 figures supporting informations

Country
France
Keywords

fano-resonant aluminum, [PHYS.PHYS.PHYS-OPTICS] Physics [physics]/Physics [physics]/Optics [physics.optics], [PHYS.PHYS.PHYS-OPTICS]Physics [physics]/Physics [physics]/Optics [physics.optics], Condensed Matter - Mesoscale and Nanoscale Physics, FOS: Physical sciences, plasmonic materials, nanoplasmonics, gold, nanoprisms, nanoantennas, ultraviolet, nanostructures, Mesoscale and Nanoscale Physics (cond-mat.mes-hall), nanoparticles, conversion, [PHYS.COND]Physics [physics]/Condensed Matter [cond-mat], [PHYS.COND] Physics [physics]/Condensed Matter [cond-mat]

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    popularity
    This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
    Top 10%
    influence
    This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
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    impulse
    This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
11
Top 10%
Average
Top 10%
Green