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Hyperuniform Monocrystalline Structures by Spinodal Solid-State Dewetting

Authors: Marco Salvalaglio; Mohammed Bouabdellaoui; Monica Bollani; Abdennacer Benali; Luc Favre; Jean-Benoit Claude; Jerome Wenger; +4 Authors

Hyperuniform Monocrystalline Structures by Spinodal Solid-State Dewetting

Abstract

Materials featuring anomalous suppression of density fluctuations over large length scales are emerging systems known as disordered hyperuniform. The underlying hidden order renders them appealing for several applications, such as light management and topologically protected electronic states. These applications require scalable fabrication, which is hard to achieve with available top-down approaches. Theoretically, it is known that spinodal decomposition can lead to disordered hyperuniform architectures. Spontaneous formation of stable patterns could thus be a viable path for the bottom-up fabrication of these materials. Here we show that mono-crystalline semiconductor-based structures, in particular Si$_{1-x}$Ge$_{x}$ layers deposited on silicon-on-insulator substrates, can undergo spinodal solid-state dewetting featuring correlated disorder with an effective hyperuniform character. Nano- to micro-metric sized structures targeting specific morphologies and hyperuniform character can be obtained, proving the generality of the approach and paving the way for technological applications of disordered hyperuniform metamaterials. Phase-field simulations explain the underlying non-linear dynamics and the physical origin of the emerging patterns.

6 pages, 3 figures, supplementary information (7 pages) enclosed

Countries
Italy, France, Italy, Italy
Keywords

Condensed Matter - Materials Science, hyper-unifom, Materials Science (cond-mat.mtrl-sci), FOS: Physical sciences, spinodal, hyper uniform, [PHYS] Physics [physics], spinodal material, Disordered Hyperuniform metamaterials, Semiconductor, dewetting, phase field simulation, SiGe dewetted

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selected citations
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This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
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