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ZENODO
Dataset . 2021
License: CC BY
Data sources: Datacite
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ZENODO
Dataset . 2021
License: CC BY
Data sources: ZENODO
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ZENODO
Dataset . 2021
License: CC BY
Data sources: Datacite
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Smithsonian figshare
Dataset . 2021
License: CC BY
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Measurement report: quantifying source contribution of fossil fuels and biomass-burning black carbon aerosol in the southeastern margin of the Tibetan Plateau

Authors: Huikun Liu (758530); Qiyuan Wang (434809); Li Xing (35790); Yong Zhang (5893); Ting Zhang (102583); Weikang Ran (7475111); Junji Cao (434810);

Measurement report: quantifying source contribution of fossil fuels and biomass-burning black carbon aerosol in the southeastern margin of the Tibetan Plateau

Abstract

Anthropogenic emissions of Black carbon (BC) aerosol are transported from Southeast Asia to the southwestern Tibetan Plateau (TP) during the pre-monsoon; however, the quantities of BC from different anthropogenic sources and the transport mechanisms are still not well constrained because there have been no high-time-resolution BC source apportionments. Intensive measurements were taken in a transport channel for pollutants from Southeast Asia to the southeastern margin of TP during the pre-monsoon to investigate the influences of fossil fuels and biomass burning on BC. A receptor model coupled multi-wavelength absorption with aerosol species concentrations was used to retrieve site-specific Ångström exponents (AAE) and mass absorption cross-sections (MAC) for BC. An ‘aethalometer model’ that used those values showed that biomass burning had a larger contribution to BC mass than fossil fuels (BCbiomass = 57% versus BCfossil = 43%). The potential source contribution function indicated that BCbiomass was transported to the site from northeastern India and northern Burma, The Weather Research and Forecasting model coupled with chemistry (WRF-Chem) model indicated that 40% of BCbiomass originated from Southeast Asia, while the high BCfossil was transported from the southwest of sampling site. A radiative transfer model indicated that the average atmospheric direct radiative effects (DRE) of BC was +4.6 ± 2.4 W m-2 with +2.5 ± 1.8 W m-2 from BCbiomass and +2.1 ± 0.9 W m-2 from BCfossil. The DRE of BCbiomass and BCfossil produced heating rates of 0.07 ± 0.05 and 0.06 ± 0.02 K day-1, respectively. This study provides insights into sources of BC over a transport channel to the southeastern TP and the influence of the cross-border transportation of biomass burning emissions from Southeast Asia during the pre-monsoon.

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Keywords

TP, Chemical Sciences not elsewhere classified, mass absorption cross-sections, Biophysics, high-time-resolution BC source appo., Biochemistry, 0.9 W m -2, source contribution function, transport channel, Sociology, Tibetan Plateau Anthropogenic emissions, quantifying source contribution, Environmental Sciences not elsewhere classified, Genetics, BCbiomas, AAE, plusmn, radiative transfer model, 2.4 W m -2, Cancer, MAC, Ecology, 1.8 W m -2, aerosol species concentrations, DRE, biomas, Southeast Asia, Astronomical and Space Sciences not elsewhere classified, BCfossil, pre-monsoon, 0.02 K day, Biological Sciences not elsewhere classified

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selected citations
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This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
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popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
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influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
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impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
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