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Orbital Angular Momentum and Energy Loss Characterization of Plasmonic Excitations in Metallic Nanostructures in TEM

Authors: Zanfrognini M; Rotunno E; Frabboni S; Sit A; Karimi E; Hohenester U; Grillo V;

Orbital Angular Momentum and Energy Loss Characterization of Plasmonic Excitations in Metallic Nanostructures in TEM

Abstract

Recently, a new device to measure the Orbital Angular Momentum (OAM) electronic spectrum after elastic/inelastic scattering in a transmission electron microscope has been introduced. We modified the theoretical framework needed to describe conventional low loss electron energy loss spectroscopy (EELS) experiments in transmission electron microscopes (TEM) to study surface plasmons in metallic nanostructures, to allow for an OAM post selection and devise new experiments for the analysis of these excitations in nanostructures. We found that unprecedented information on the symmetries and on the chirality of the plasmonic modes can be retrieved even with limited OAM and energy resolutions.

Country
Italy
Keywords

---, EELS, Physics - Instrumentation and Detectors, Orbital angular momentum, FOS: Physical sciences, Instrumentation and Detectors (physics.ins-det), electron beam shaping, plasmonics; electron energy loss spectroscopy; electron orbital angular momentum; transmission electron microscopy, plasmon modes, Physics - Optics, Optics (physics.optics)

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selected citations
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This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
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