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We present a tunnel spectroscopy study of single PbS Quantum Dots (QDs) as function of temperature and gate voltage. Three distinct signatures of strong electron-phonon coupling are observed in the Electron Tunneling Spectrum (ETS) of these QDs. In the shell-filling regime, the $8\times$ degeneracy of the electronic levels is lifted by the Coulomb interactions and allows the observation of phonon sub-bands that result from the emission of optical phonons. At low bias, a gap is observed in the ETS that cannot be closed with the gate voltage, which is a distinguishing feature of the Franck-Condon (FC) blockade. From the data, a Huang-Rhys factor in the range $S\sim 1.7 - 2.5$ is obtained. Finally, in the shell tunneling regime, the optical phonons appear in the inelastic ETS $d^2I/dV^2$.
5 pages, 5 figures
[CHIM.MATE] Chemical Sciences/Material chemistry, Condensed Matter - Mesoscale and Nanoscale Physics, tunnel spectroscopy, Mesoscale and Nanoscale Physics (cond-mat.mes-hall), quantum dot, FOS: Physical sciences, PbS, [PHYS.COND] Physics [physics]/Condensed Matter [cond-mat]
[CHIM.MATE] Chemical Sciences/Material chemistry, Condensed Matter - Mesoscale and Nanoscale Physics, tunnel spectroscopy, Mesoscale and Nanoscale Physics (cond-mat.mes-hall), quantum dot, FOS: Physical sciences, PbS, [PHYS.COND] Physics [physics]/Condensed Matter [cond-mat]
citations This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically). | 16 | |
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influence This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically). | Average | |
impulse This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network. | Top 10% |