Powered by OpenAIRE graph
Found an issue? Give us feedback
image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/ Acta Physica Sinicaarrow_drop_down
image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
Acta Physica Sinica
Article . 2019 . Peer-reviewed
Data sources: Crossref
image/svg+xml art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos Open Access logo, converted into svg, designed by PLoS. This version with transparent background. http://commons.wikimedia.org/wiki/File:Open_Access_logo_PLoS_white.svg art designer at PLoS, modified by Wikipedia users Nina, Beao, JakobVoss, and AnonMoos http://www.plos.org/
Acta Physica Sinica
Article
License: CC BY
Data sources: UnpayWall
versions View all 1 versions
addClaim

This Research product is the result of merged Research products in OpenAIRE.

You have already added 0 works in your ORCID record related to the merged Research product.

Theoretical study of dissociation dynamics of HD<sup>+</sup> and its quantum control with an intense laser field

Authors: Hong-Bin Yao; Xiang-Zhan Jiang; Chang-Hong Cao; Wen-Liang Li;

Theoretical study of dissociation dynamics of HD<sup>+</sup> and its quantum control with an intense laser field

Abstract

The dissociation dynamics of HD<sup>+</sup> molecule in an intense field is investigated by using an accurate three-dimensional time-dependent wave packet approach. When the 790-nm laser pulse interacts with HD<sup>+</sup> molecule, the lowest electronic 1sσ and 2pσ states are coupled. Due to the existence of the permanent electric dipole moment, the transitions in HD<sup>+</sup> molecule involve the direct absorption of an odd and even number of photons, thereby opening different pathways for dissociation. The model of the photon-dressed states is presented to analyze the possible dissociation pathways of HD<sup>+</sup> molecule. The laser-induced dissociation of HD<sup>+</sup> molecule is mainly composed of the four pathways: the direct one-photon absorption, the net two-photon absorption, the direct two-photon absorption, and the direct two-photon absorption. To reveal the dissociation mechanism of HD<sup>+</sup> molecule, the kinetic energy resolved spectra are calculated at the given laser intensities. It is found that the dissociation pathways are strongly dependent on laser intensity, especially for the net one-photon absorption dissociation and direct two-photon absorption dissociation. With further research, the dissociation pathways of HD<sup>+</sup> are controlled by regulating the intensity of laser pulse. At a laser intensity of 4.0 × 10<sup>13</sup> W/cm<sup>2</sup>, the kinetic energy resolved spectrum for the vibrational state <i>ν</i> = 3 includes the contributions from the net two-photon absorption dissociation and the direct two-photon absorption dissociation. For the vibrational state <i>ν</i> = 6, HD<sup>+</sup> molecule is preferentially dissociated via the net one-photon absorption. However, the dissociation mechanism of HD<sup>+</sup> molecule at the vibrational states <i>ν</i> = 3 and <i>ν</i> = 6 have significant changes as the laser intensity increases to 2.0 × 10<sup>14</sup> W/cm<sup>2</sup>. For the vibrational state <i>ν</i> = 3, the branching ratio between the dissociation pathway of the net two-photon absorption and that of the direct two-photon absorption has a dramatic change with the increase of laser intensity. Compared with the kinetic energy resolved spectra at laser energy of 4.0 × 10<sup>13</sup> W/cm<sup>2</sup>, the height of the dissociation peak from the net two-photon absorption decreases, and that of the direct two-photon absorption increases at laser intensity of 2.0 × 10<sup>14</sup> W/cm<sup>2</sup>. For the vibrational state <i>ν</i> = 6, the dissociation process of the net one-photon absorption almost disappears at laser intensity of 2.0 × 10<sup>14</sup> W/cm<sup>2</sup>, and it is replaced by the dissociation pathway of the direct two-photon absorption.

  • BIP!
    Impact byBIP!
    selected citations
    These citations are derived from selected sources.
    This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
    0
    popularity
    This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
    Average
    influence
    This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
    Average
    impulse
    This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
    Average
Powered by OpenAIRE graph
Found an issue? Give us feedback
selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
0
Average
Average
Average
gold