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Large‐Area Synthesis of Ferromagnetic Fe5−xGeTe2/Graphene van der Waals Heterostructures with Curie Temperature above Room Temperature

Authors: Lv, Hua; da Silva, Alessandra; Figueroa, Adriana I.; Guillemard, Charles; Aguirre, Iván Fernández; Camosi, Lorenzo; Aballe, Lucia; +10 Authors

Large‐Area Synthesis of Ferromagnetic Fe5−xGeTe2/Graphene van der Waals Heterostructures with Curie Temperature above Room Temperature

Abstract

AbstractVan der Waals (vdW) heterostructures combining layered ferromagnets and other 2D crystals are promising building blocks for the realization of ultracompact devices with integrated magnetic, electronic, and optical functionalities. Their implementation in various technologies depends strongly on the development of a bottom‐up scalable synthesis approach allowing for realizing highly uniform heterostructures with well‐defined interfaces between different 2D‐layered materials. It is also required that each material component of the heterostructure remains functional, which ideally includes ferromagnetic order above room temperature for 2D ferromagnets. Here, it is demonstrated that the large‐area growth of Fe5−xGeTe2/graphene heterostructures is achieved by vdW epitaxy of Fe5−xGeTe2 on epitaxial graphene. Structural characterization confirms the realization of a continuous vdW heterostructure film with a sharp interface between Fe5−xGeTe2 and graphene. Magnetic and transport studies reveal that the ferromagnetic order persists well above 300 K with a perpendicular magnetic anisotropy. In addition, epitaxial graphene on SiC(0001) continues to exhibit a high electronic quality. These results represent an important advance beyond nonscalable flake exfoliation and stacking methods, thus marking a crucial step toward the implementation of ferromagnetic 2D materials in practical applications.

Countries
Germany, France, Spain, Spain, Germany
Keywords

Condensed Matter - Materials Science, van der Waals epitaxy, graphene, Materials Science (cond-mat.mtrl-sci), FOS: Physical sciences, Fe5−xGeTe2, Physics - Applied Physics, Applied Physics (physics.app-ph), [PHYS.COND.CM-MS] Physics [physics]/Condensed Matter [cond-mat]/Materials Science [cond-mat.mtrl-sci], 620, 2D spintronics, 2D magnets, van der Waals heterostructures, info:eu-repo/classification/ddc/620

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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
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