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Physical Review Letters
Article . 2021 . Peer-reviewed
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https://dx.doi.org/10.48550/ar...
Article . 2020
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Disentangling Orbital and Valley Hall Effects in Bilayers of Transition Metal Dichalcogenides

Authors: Tarik P. Cysne; Marcio Costa; Luis M. Canonico; M. Buongiorno Nardelli; R. B. Muniz; Tatiana G. Rappoport;

Disentangling Orbital and Valley Hall Effects in Bilayers of Transition Metal Dichalcogenides

Abstract

It has been recently shown that monolayers of transition metal dichalcogenides (TMDs) in the 2H structural phase exhibit relatively large orbital Hall conductivity plateaus within their energy band gaps, where their spin Hall conductivities vanish. However, since the valley Hall effect (VHE) in these systems also generates a transverse flow of orbital angular momentum it becomes experimentally challenging to distinguish between the two effects in these materials. The VHE requires inversion symmetry breaking to occur, which takes place in the TMD monolayers, but not in the bilayers. We show that a bilayer of 2H-MoS$_2$ is an orbital Hall insulator that exhibits a sizeable OHE in the absence of both spin and valley Hall effects. This phase can be characterised by an orbital Chern number that assumes the value $\mathcal{C}_{L}=2$ for the 2H-MoS$_2$ bilayer and $\mathcal{C}_{L}=1$ for the monolayer, confirming the topological nature of these orbital-Hall insulator systems. Our results are based on density functional theory (DFT) and low-energy effective model calculations and strongly suggest that bilayers of TMDs are highly suitable platforms for direct observation of the orbital Hall insulating phase in two-dimensional materials. Implications of our findings for attempts to observe the VHE in TMD bilayers are also discussed.

7 pages, 4 figures + Supplementary material

Countries
Spain, United States
Keywords

spintronics, atomic orbitals, Condensed Matter - Mesoscale and Nanoscale Physics, Direct observations, Orbital angular momentum, Hall effect, FOS: Physical sciences, Spintronics, Spin hall conductivity, Two-dimensional materials, Transition metal dichalcogenides, Valleytronics, Mesoscale and Nanoscale Physics (cond-mat.mes-hall), valleytronics, Inversion symmetry, Model calculations, Hall conductivity, Atomic orbital

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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
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