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Narrow Line Width Quantum Emitters in an Electron-Beam-Shaped Polymer

Authors: Pietro Lombardi; Alessandro Lavacchi; Camilla Dore; Sofia Pazzagli; Wolfram H. P. Pernice; Carlotta Ciancico; Maja Colautti; +9 Authors

Narrow Line Width Quantum Emitters in an Electron-Beam-Shaped Polymer

Abstract

Solid-state single photon sources (SPSs) with narrow line width play an important role in many leading quantum technologies. Within the wide range of SPSs studied to date, single fluorescent molecules hosted in organic crystals stand out as bright, photostable SPSs with a lifetime-limited optical resonance at cryogenic temperatures. Furthermore, recent results have demonstrated that photostability and narrow line widths are still observed from single molecules hosted in a nanocrystalline environment, which paves the way for their integration with photonic circuitry. Polymers offer a compatible matrix for embedding nanocrystals and provide a versatile yet low-cost approach for making nanophotonic structures on chip that guide light and enhance coupling to nanoscale emitters. Here, we present a deterministic nanostructuring technique based on electron-beam lithography for shaping polymers with embedded single molecules. Our approach provides a direct means of structuring the nanoscale environment of narrow line width emitters while preserving their emission properties.

Countries
Italy, Spain
Keywords

Condensed Matter - Mesoscale and Nanoscale Physics, Single molecule, Quantum emitters, FOS: Physical sciences, Physics - Applied Physics, Applied Physics (physics.app-ph), Single photon source quantum emitters, single molecule electron beam lithography, On-chip quantum optics, Single photon source, on-chip quantum optics, Mesoscale and Nanoscale Physics (cond-mat.mes-hall), Electron beam lithography, nanophotonic devices, Nanophotonic devices

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download
citations
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
views
OpenAIRE UsageCountsViews provided by UsageCounts
downloads
OpenAIRE UsageCountsDownloads provided by UsageCounts
9
Top 10%
Average
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35
71
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bronze