ABSTRACTHighly-uniform, hollow glass spheres, which are used for inertial-confinement fusion targets, are formed from metalorganic gel powder feedstock in a drop-tower furnace. The modelling of this gel-to-sphere transformation has consisted of three phases: gel thermochemistry, furnace-to-gel heat transfer, and gravity-driven degradation of the concentricity of the molten shell.The heat transfer from the furnace to the free-falling gel particle was modelled with forced convection. The gel mass, dimensions, and specific heat as well as furnace temperature profile and furnace gas conductivity, were controlled variables. This model has been experimentally verified. In the third phase, a mathematical model was developed to describe the gravity-driven degradation of concentricity in molten glass shells.