AbstractNeutrons from collisions of cosmic rays with the nuclei of atoms in the atmosphere are an irremovable external radiation that causes single-event upsets in microelectronic devices. Predicting soft error rates requires knowledge of the flux and energy distribution of the cosmic-ray-induced neutrons. This article reviews cosmic-ray neutrons in the atmosphere and on the ground, the factors that determine their intensity, and recent calculations and state-of-the-art measurements of neutron spectra covering 12 decades of energy, from the thermal energy range up to 10 GeV.