In this paper, we experimentally study transient dynamics of spin polarized atoms in the spin-exchange-relaxation-free (SERF) regime with a single-beam configuration. We pumped atoms with a weak detuning pumping beam, along with a sequence of magnetic field pulses orthogonal to the pumping beam were applied. The dynamics of atomic spin, which experiences Larmor precession under the perturbation of magnetic field, is detected by the transmitted pumping beam. Benefited from the long coherence time of atomic spin in the SERF regime, the dependence of precession frequency and decay rate, which is equal to the magnetic resonance linewidth of atomic spin, on magnetic fields is studied with the transient dynamics of atomic spin in the limit of low spin polarization. Moreover, we demonstrate that coil constants can be calibrated by analyzing the precession frequency of the transient dynamics of atomic spin. And the experimental results show that the coil constants are 114.25 ± 0.02 nT/mA and 114.12 ± 0.04 nT/mA in x- and y-axis, respectively. This method is particularly applicable to study the atomic spin dynamics and calibrate the coil constant in situ of a miniature single-beam SERF magnetometer.