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https://doi.org/10.1103/physre...
Article . 2017 . Peer-reviewed
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https://dx.doi.org/10.48550/ar...
Article . 2017
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Charge transport in hybrid halide perovskites

Authors: Zhang, Mingliang; Zhang, Xu; Huang, Ling-Yi; Lin, Hai-Qing; Lu, Gang;

Charge transport in hybrid halide perovskites

Abstract

Charge transport is crucial to the performance of hybrid halide perovskite solar cells. A theoretical model based on large polarons is proposed to elucidate charge transport properties in the perovskites. Critical new physical insights are incorporated into the model, including the recognitions that acoustic phonons as opposed to optical phonons are responsible for the scattering of the polarons; these acoustic phonons are fully excited due to the "softness" of the perovskites, and the temperature-dependent dielectric function underlies the temperature dependence of charge carrier mobility. This work resolves key controversies in literature and forms a starting point for more rigorous first-principles predictions of charge transport.

9 figures, 15 pages, accepted by Phys. Rev. B

Keywords

Condensed Matter - Materials Science, Materials Science (cond-mat.mtrl-sci), FOS: Physical sciences

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    popularity
    This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
    Top 10%
    influence
    This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
    Top 10%
    impulse
    This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
24
Top 10%
Top 10%
Top 10%
Green
hybrid