
A significant part of the cost for carbon capture and storage (CCS) is related to the compression of captured CO2 to its supercritical state, at 150 bar and typically 99% purity. These stringent conditions may however not always be necessary for specific cases of carbon capture and utilization (CCU). In this manuscript, we investigate how much the parasitic energy of an adsorbent-based carbon capture process may be lowered by utilizing CO2 at 1 bar and adapting the final purity requirement for CO2 from 99% to 70% or 50%. We compare different CO2 sources: the flue gases of coal-fired or natural gas-fired power plants and ambient air. We evaluate the carbon capture performance of over 60 nanoporous materials and determine the influence of the initial and final CO2 purity on the parasitic energy of the carbon capture process. Moreover, we demonstrate the underlying principles of the parasitic energy minimization in more detail using the commercially available NaX zeolite. Finally, the calculated utilization cost of CO2 is compared with the reported prices for CO2 and published costs for CCS.
MOLECULAR SIMULATION, Chemical Physics, GAS-ADSORPTION, ZEOLITIC IMIDAZOLATE FRAMEWORKS, POROUS POLYMER NETWORKS, CU-BTC, Climate Action, Chemistry, METAL-ORGANIC FRAMEWORKS, Affordable and Clean Energy, PRESSURE-SWING ADSORPTION, Chemical Sciences, DIRECT AIR CAPTURE, CO2 CAPTURE, DIOXIDE CAPTURE
MOLECULAR SIMULATION, Chemical Physics, GAS-ADSORPTION, ZEOLITIC IMIDAZOLATE FRAMEWORKS, POROUS POLYMER NETWORKS, CU-BTC, Climate Action, Chemistry, METAL-ORGANIC FRAMEWORKS, Affordable and Clean Energy, PRESSURE-SWING ADSORPTION, Chemical Sciences, DIRECT AIR CAPTURE, CO2 CAPTURE, DIOXIDE CAPTURE
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