
doi: 10.1021/ef5023779
handle: 11583/2598765
This work focuses on the process design and performance of an innovative plant for digester gas upgrading to synthetic natural gas (SNG). The differences and advantages over traditional upgrading processes are discussed. The main strength of digester gas upgrading via high-temperature electrolysis concerns its higher synthetic natural gas productivity for a given raw digester gas feed. Electrolysis is performed through a solid oxide electrolysis cell (SOEC) system, which is fed with demineralized water and purified digester gas (made up of methane and carbon dioxide). Surplus electricity from intermittent renewable energy sources is used to supply the energy required for the SOEC stacks. The resulting methane-rich syngas is reacted in a series of methanators to yield a high CH4 content output stream. The steam reforming reaction is promoted by means of a nickel catalyst in the cathode (fuel) electrode, which reduces the methane fraction: hence, sulfur, which is present in several types of digester gas (e....
Engineering controlled terms: Air purification; Anaerobic digestion; Biogas; Carbon; Carbon dioxide; Catalysts; Electrodes; Electrolysis; Electrolytic cells; Gases; Methane; Natural gas; Renewable energy resources; Sewage; Solid oxide fuel cells (SOFC); Steam reforming; Sulfur Biological substrates; Demineralized water; Electrochemical performance; High temperature electrolysis; Renewable energy source; Solid oxide electrolysis cells; Synthetic natural gas; Thermodynamic conditions
Engineering controlled terms: Air purification; Anaerobic digestion; Biogas; Carbon; Carbon dioxide; Catalysts; Electrodes; Electrolysis; Electrolytic cells; Gases; Methane; Natural gas; Renewable energy resources; Sewage; Solid oxide fuel cells (SOFC); Steam reforming; Sulfur Biological substrates; Demineralized water; Electrochemical performance; High temperature electrolysis; Renewable energy source; Solid oxide electrolysis cells; Synthetic natural gas; Thermodynamic conditions
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