The problem of low material utilization caused by premature interface debonding is prevalent in carbon fiber-reinforced polymer (CFRP)-reinforced concrete structures. In this study, the influence of anchors on the bonding and behavior of the FRP-engineered cementitious composite (ECC) layer and concrete interface was analyzed. A total of 42 single shear tests were performed to investigate the interface–bond behavior between the FRP-ECC layer and concrete under static load in case of anchor reinforcement. The variables mainly include the matrix type, anchor location, anchor spacing, and number of anchors. The results show that the anchor can increase the interfacial load-carrying capacity up to 85%; the maximum slip value of the interface can also be enhanced. Furthermore, the influence of the location, spacing, and number of anchors on the interface bonding performance is closely related to the effective bonding length and post-anchor bond length. The effective bonding length is 400 mm based on the strain distribution calculation and analysis. The test results provide valuable information for FRP anchor reinforcement in FRP-ECC composite layer-reinforced concrete structures. © 2024 Elsevier Ltd