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Optical luminescence of electronic and vibronic transitions in Gd2−xYx(SO4)3 · 8H2O

descriptionPublicationkeyboard_double_arrow_right Article 01 Mar 1990 English Publisher:Elsevier BVJournal:Journal of Solid State Chemistry, volume 85, pages 1-7 (issn: 0022-4596,

Authors: M.K. Crawford; L.H. Brixner; G. Blasse;

doi: 10.1016/s0022-4596(05)80052-0

Optical luminescence of electronic and vibronic transitions in Gd2−xYx(SO4)3 · 8H2O

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Abstract

Abstract X-ray and ultraviolet-excited emission spectra of Gd 2 (SO 4 ) 3 · 8H 2 O show the electronic 6 P 3/2,5/2,7/2, → 8 S 7/2, lines of Gd 3+ accompanied by vibronics involving the water and sulfate vibrations. Removal of the water of hydration by heating eliminates the water vibronics, while the spectrum of Gd 2 (SO 4 ) 3 · 8D 2 O exhibits the expected shift toward the electronic origin of vibronics attributed to the water of hydration. In a dilute system of composition Gd 0.8 Y 1.2 (SO 4 ) 3 · 8H 2 O we also see the 6 D J , 6 I J → 8 S 7/2 level transitions.

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