
The first two experimental chapters of this report have focused on the design and exploration of semiconducting transition metal dichalcogenide-based quantum dots (TMD-QDs) as single-photon sources. This chapter presents the first efforts in using TMD-QDs as matter qubits, by electrically capturing a single charge inside the QDs. This charge will occupy a quantum state (e.g. spin or valley pseudospin) which can be used to store quantum information and perform computations via optical excitation [1].
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