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image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao ChemSusChemarrow_drop_down
image/svg+xml Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao Closed Access logo, derived from PLoS Open Access logo. This version with transparent background. http://commons.wikimedia.org/wiki/File:Closed_Access_logo_transparent.svg Jakob Voss, based on art designer at PLoS, modified by Wikipedia users Nina and Beao
ChemSusChem
Article . 2024 . Peer-reviewed
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All‐in‐All: Dead Lithium‐Ion Battery to Active Lithium‐Ion Capacitor

Authors: Akshay Manohar; Aranganathan Viswanathan; Yun‐Sung Lee; Vanchiappan Aravindan;

All‐in‐All: Dead Lithium‐Ion Battery to Active Lithium‐Ion Capacitor

Abstract

AbstractHere, we have developed lithium‐ion capacitors (LICs) with all the components, except the electrolyte solution, effectively recycled from the spent Lithium‐ion batteries (LIBs). Hybrid capacitors, such as LICs, are potential breakthroughs in electrochemical energy storage devices, where most research is focused. These devices can simultaneously guarantee high energy and power by hybridizing battery‐type and capacitive‐type electrodes with two different reaction mechanisms. We have successfully upcycled the graphite, current collector, separator, etc., from the spent LIBs to fabricate a high‐performance LIC. Our LIC consists of recovered graphite (RG) coated over recovered copper foil as an anode, recycled polypropylene as the separator, and reduced graphene oxide (rGO) synthesized from RG as the cathode. The RG half‐cell exhibited an excellent specific capacity of 302 mAh g−1 even after 75 charge‐discharge cycles with a coulombic efficiency of >99 %. The Li/rGO displayed remarkable cycling performance for over 1000 cycles with high stability and reversibility. Subsequently, the pre‐lithiated RG (p‐RG) electrode is paired with the rGO electrode under the balanced loading conditions to construct LIC, rGO/p‐RG, delivering a maximum energy density of 185 Wh kg−1 with ultra‐long durability of more than 10,000 cycles. The possibility of LIC under different climatic conditions is also explored, and its remarkable performance under various temperature conditions is worth mentioning.

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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
8
Top 10%
Average
Top 10%
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