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Weak and Strong Coupling Properties of Surface Excitons

Authors: Arpan Dutta; J. Jussi Toppari;

Weak and Strong Coupling Properties of Surface Excitons

Abstract

With high enough doping concentrations organic dye doped polymer materials exhibit negative real part of the permittivity within an energy range just above their material absorption, incurring surface exciton modes at these energies. Here, we report how such modes can be used to realize strong light-matter coupling with photoactive molecules. Our simulations reveal that surface excitons can facilitate strong coupling in terms of induced transparency, however, the polaritons may not be visible in the absorption since they can easily be located outside of the narrow negative permittivity regime. Moreover, we show that the surface exciton modes cannot couple strongly with the surface plasmons. Our findings shed light on the weak and strong coupling properties of surface excitons.

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Keywords

nanorakenteet, pintailmiöt, Nanoscience Center, optiset ominaisuudet, polymeerit, kvasihiukkaset

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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
0
Average
Average
Average
hybrid