The dataset here contains the raw data and pulse programs used for the publication "Sensitivity-enhanced multidimensional solid-state NMR spectroscopy by optimal-control-based transverse mixing sequences" submitted to JACS. All data is in a native Bruker TopSpin format. Data is organized in folders corresponding to Figures of the original publication. Detailed description is included in the file description.txt. We reccomend to visit our website optimal-nmr.net for additional information about optimal control methods applied to pulse sequence development for solid-state magic-angle-spinning NMR studies of proteins.

This work was supported by the joined project of the German Research Foundation and the Czech Science Foundation (Re/1435-20 and 20-00166J, respectively), and additionally by the Helmholtz-Gemeinschaft. Computational resources were supplied by the Leibniz Supercomputing Centre (Munich), and the project "e-Infrastruktura CZ" (e-INFRA CZ LM2018140) supported by MEYS CR. We also acknowledge CF NMR of CIISB, Instruct-CZ Centre, supported by MEYS CR (LM2018127) and European Regional Development Fund-Project "UP CIISB" (No. CZ.02.1.01/0.0/0.0/18_046/0015974).