You can find here the two TimeResolved ARPES datasets used in the paper titled "Optical manipulation of Rashba-split 2-Dimensional Electron Gas". https://www.nature.com/articles/s41467-022-30742-5 Data are in Igor Pro binary format. RawData_1 is the dataset used in Fig.3. The x scaling has been converted from angle to momentum and the energy is rescaled with respect to the chemical potential at negative delays. The Time Delay scaling is found in timewave_1. Similarly, RawData_2, RawData_20 and timewave_2 are the datasets used in Fig.2 of the paper. This x scale in both datasets has been converted from angle to momentum. The y-axes in RawData_20 is the kinetic energy. The y-axes in RawData_2 is the energy rescaled to the chemical potential at each time delay. The chemical potential is obtained by fitting the topological surface state around its Fermi momentum.