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Cold and Hot Spots: From Inhibition to Enhancement by Nanoscale Phase Tuning of Optical Nanoantennas

Authors: NIcola Palombo Blascetta; Pietro Lombardi; Costanza Toninelli; Niek van Hulst;

Cold and Hot Spots: From Inhibition to Enhancement by Nanoscale Phase Tuning of Optical Nanoantennas

Abstract

Optical nanoantennas are well-known for the confinement of light into nanoscale hot spots, suitable for emission enhancement and sensing applications. Here, we show how control of the antenna dimensions allows tuning the local optical phase, hence turning a hot spot into a cold spot. We manipulate the local intensity exploiting the interference between driving and scattered field. Using single molecules as local detectors, we experimentally show the creation of subwavelength pockets with full suppression of the driving field. Remarkably, together with the cold excitation spots, we observe inhibition of emission by the phase-tuned nanoantenna. The fluorescence lifetime of a molecule scanned in such volumes becomes longer, showing slow down of spontaneous decay. In conclusion, the spatial phase of a nanoantenna is a powerful knob to tune between enhancement and inhibition in a 3-dimensional subwavelength volume.

Countries
Spain, Spain, Italy
Keywords

:Física [Àrees temàtiques de la UPC], local density of states, Àrees temàtiques de la UPC::Física, near field interference, hot spot - cold spot, single molecule, plasmonics, nanoantennas, local phase, nanoantenna, inhibition of emission, Antenes, superresolution, antenna enhancement

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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
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