Dataset files for DeepH-hybrid, containing structures and preprocessed Hamiltonian matrices computed with HSE06 hybrid functional and ABACUS DFT package. Enclosed include: The four datasets corresponding to the four DeepH-hybrid models mentioned in DeepH-hybrid's paper, each containing material structures and electronic structure properties of Basis set files for the ABACUS DFT package Snapshot of a version of the additional codes utilized to preprocess hybrid DFT Hamiltonians (also available via this GitHub link) Note only the additional codes of DeepH-hybrid is provided, and it may be used in combination with DeepH-E3 package for neural-network training. For additional details please refer to the "README" file of the code.