This dataset contains outputs from the DYAMOND Phase-II simulations, focusing on Global Storm-Resolving Models (GSRMs) at various Atmospheric Radiation Measurement (ARM) sites. The dataset supports the analysis presented in the manuscript "Boundary-Layer-Coupled and Decoupled Clouds in Global Storm-Resolving Models: Comparisons with the ARM Observations." Included are high-resolution model outputs from nine GSRMs, detailing simulations of atmospheric processes at six ARM sites, including variables of clouds, temperature, humidity, wind, and surface fluxes. This dataset allows for a direct comparison between GSRM simulations and ARM field observations, facilitating the evaluation of PBL-coupled and decoupled clouds. For further inquiries or assistance regarding the dataset, please contact the corresponding author at su10@llnl.gov.