In this volume of the EOS MLS Calibration Report we expand on the data presented in Volume 1, covering the following: Radiometric performance and calibrations, relative sideband response, FOV calibrations, and additional details of the controllers used in radiometric and spectral calibrations. We also include additional information on the locations of the calibration data files, and some of the software used to create them. Volume 3 of this report is devoted to presentation of the voluminous high-resolution spectral sweep data, and Volume 4 to post-launch updates to instrument performance and calibrations.