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Experimental observation of the liquid-liquid transition in bulk supercooled water under pressure

Authors: Kyung Hwan Kim; Katrin Amman-Winkel; Nicolas Giovambattista; Alexander Späh; Fivos Perakis; Harshad Pathak; Marjorie Ladd Parada; +14 Authors
APC: 3,510.7 EUR

Experimental observation of the liquid-liquid transition in bulk supercooled water under pressure

Abstract

Liquid-liquid transitions under pressure Theoretical simulations suggest that deeply supercooled water undergoes a transition between high- and low-density forms, but this transition is difficult to study experimentally because it occurs under conditions in which ice crystallization is extremely rapid. Kim et al. combined x-ray lasers for rapid structure determination with infrared femtosecond pulses for rapid heating of amorphous ice layers formed at about 200 kelvin. The heating process created high-density liquid water at increased pressures. As the layer expanded and decompressed, low-density liquid domains appeared and grew on time scales between 20 nanoseconds and 3 microseconds, which was much faster than competing ice crystallization. Science , this issue p. 978

Countries
Korea (Republic of), Germany
Keywords

DYNAMICS, info:eu-repo/classification/ddc/320, ICE, SINGULARITY, LASER, ELECTRON, CRYSTALLIZATION, HIGH-DENSITY, 320

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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
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OpenAIRE UsageCountsViews provided by UsageCounts
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bronze