Abstract Context In a large object-oriented software system, packages play the role of modules which group related classes together to provide well-identified services to the rest of the system. In this context, it is widely believed that modularization has a large influence on the quality of packages. Recently, Sarkar, Kak, and Rama proposed a set of new metrics to characterize the modularization quality of packages from important perspectives such as inter-module call traffic, state access violations, fragile base-class design, programming to interface, and plugin pollution. These package-modularization metrics are quite different from traditional package-level metrics, which measure software quality mainly from size, extensibility, responsibility, independence, abstractness, and instability perspectives. As such, it is expected that these package-modularization metrics should be useful predictors for fault-proneness. However, little is currently known on their actual usefulness for fault-proneness prediction, especially compared with traditional package-level metrics. Objective In this paper, we examine the role of these new package-modularization metrics for determining software fault-proneness in object-oriented systems. Method We first use principal component analysis to analyze whether these new package-modularization metrics capture additional information compared with traditional package-level metrics. Second, we employ univariate prediction models to investigate how these new package-modularization metrics are related to fault-proneness. Finally, we build multivariate prediction models to examine the ability of these new package-modularization metrics for predicting fault-prone packages. Results Our results, based on six open-source object-oriented software systems, show that: (1) these new package-modularization metrics provide new and complementary views of software complexity compared with traditional package-level metrics; (2) most of these new package-modularization metrics have a significant association with fault-proneness in an expected direction; and (3) these new package-modularization metrics can substantially improve the effectiveness of fault-proneness prediction when used with traditional package-level metrics together. Conclusions The package-modularization metrics proposed by Sarkar, Kak, and Rama are useful for practitioners to develop quality software systems.