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A reactive coevaporation system for i n s i t u, epitaxial YBa2Cu3O7−x thin film deposition

Authors: Siu-Wai Chan; S. M. Sampere; L. A. Farrow; J. B. Barner; C. T. Rogers; B. J. Wilkens; E. W. Chase;

A reactive coevaporation system for i n s i t u, epitaxial YBa2Cu3O7−x thin film deposition

Abstract

A new ultrahigh vacuum system has been specially designed and built to deposit high temperature superconducting thin films over a large area with great uniformity in both thickness and composition. The sources are in close proximity and a large distance (460 mm) separates the substrate holder and the sources. We will describe the design and the capabilities of the system including the design rationale. We have prepared in situ YBa2Cu3O7−x films to demonstrate the feasibility of the system. As configured, the reactive coevaporation system can deposit up to 35 mm diam YBa2Cu3O7−x films. Evaporant uniformity is expected up to 60 mm diam with the present limit in area set by the heater size, the size of the appropriate substrates, and the difficulty in attachment of substrates to the holder with uniform thermal contact. Films are prepared by coevaporation of yttrium, barium, and copper from three different evaporation sources with the substrate holder temperature measured at 680 °C in a PO2=5×10−4 Torr ambient. Because the substrate holder is 460 mm above the sources, debris from the sources cannot travel upward and stick to the film surface. Films less than 250 nm thick on (001) SrTiO3 and (001) LaAlO3 exhibit a sharp transition width (ΔT=0.5 K) and Tc(R=0)=90 K by resistivity measurements. In addition, alternating-current (ac) magnetic susceptibility characterization shows sharp transitions (<1 K) at a slightly lower temperature implying that the induced screening current is uniform over the area of the detection coil. These films are structurally very close to single crystals as characterized by both x-ray diffraction and Raman scattering.

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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
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