
Transition-metal-based kagome materials at van Hove filling are a rich frontier for the investigation of novel topological electronic states and correlated phenomena. To date, in the idealized two-dimensional kagome lattice, topologically Dirac surface states (TDSSs) have not been unambiguously observed, and the manipulation of TDSSs and van Hove singularities (VHSs) remains largely unexplored. Here, we reveal TDSSs originating from a Z2 bulk topology and identify multiple VHSs near the Fermi level (EF) in magnetic kagome material GdV6Sn6. Using in situ surface potassium deposition, we successfully realize manipulation of the TDSSs and VHSs. The Dirac point of the TDSSs can be tuned from above to below EF, which reverses the chirality of the spin texture at the Fermi surface. These results establish GdV6Sn6 as a fascinating platform for studying the nontrivial topology, magnetism, and correlation effects native to kagome lattices. They also suggest potential application of spintronic devices based on kagome materials.
ARPES DFT, ARPES+DFT, Materials Science and Engineering, Kagome Metal GdV6Sn6, Sino-Swiss Science and Technology Cooperation, Sino Swiss Science and Technology Cooperation, TDSSs and VHSs, NCCR MARVEL
ARPES DFT, ARPES+DFT, Materials Science and Engineering, Kagome Metal GdV6Sn6, Sino-Swiss Science and Technology Cooperation, Sino Swiss Science and Technology Cooperation, TDSSs and VHSs, NCCR MARVEL
| citations This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically). | 0 | |
| popularity This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network. | Average | |
| influence This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically). | Average | |
| impulse This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network. | Average |
