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https://doi.org/10.1103/physre...
Article . 2024 . Peer-reviewed
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https://dx.doi.org/10.48550/ar...
Article . 2024
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Magnetic structure and Ising-like antiferromagnetism in the bilayer triangular lattice compound NdZnPO

Authors: Han Ge; Tiantian Li; Stanislav E. Nikitin; Nan Zhao; Fangli Li; Huanpeng Bu; Jiayue Yuan; +10 Authors

Magnetic structure and Ising-like antiferromagnetism in the bilayer triangular lattice compound NdZnPO

Abstract

The complex interplay of spin frustration and quantum fluctuations in low-dimensional quantum materials leads to a variety of intriguing phenomena. This research focuses on a detailed analysis of the magnetic behavior exhibited by NdZnPO, a bilayer spin-1/2 triangular lattice antiferromagnet. The investigation employs magnetization, specific heat, and powder neutron scattering measurements. At zero field, a long-range magnetic order is observed at $T_{\rm N}=1.64~\rm K$. Powder neutron diffraction experiments show the Ising-like magnetic moments along the $c$-axis, revealing a stripe-like magnetic structure with three equivalent magnetic propagation vectors. Application of a magnetic field along the $c$-axis suppresses the antiferromagnetic order, leading to a fully polarized ferromagnetic state above $B_{\rm c}=4.5~\rm T$. This transition is accompanied by notable enhancements in the nuclear Schottky contribution. Moreover, the absence of spin frustration and expected field-induced plateau-like phases are remarkable observations. Detailed calculations of magnetic dipolar interactions revealed complex couplings reminiscent of a honeycomb lattice, suggesting the potential emergence of Kitaev-like physics within this system. This comprehensive study of the magnetic properties of NdZnPO highlights unresolved intricacies, underscoring the imperative for further exploration to unveil the underlying governing mechanisms.

11 pages, 6 figures

Country
Spain
Keywords

Condensed Matter - Strongly Correlated Electrons, Condensed Matter - Materials Science, Strongly Correlated Electrons (cond-mat.str-el), 500, Materials Science (cond-mat.mtrl-sci), FOS: Physical sciences, 530

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popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
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influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
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impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
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