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Purification of Uranium‐based Endohedral Metallofullerenes (EMFs) by Selective Supramolecular Encapsulation and Release

descriptionPublicationkeyboard_double_arrow_right Article 26 Jul 2018 Spain English Publisher:WileyJournal:Angewandte Chemie International Edition, volume 57, pages 11,294-11,299 (issn: 1433-7851, eissn: 1521-3773, Copyright policy )Funded by:NSF | UTEP/UCSB PREM: Molecular..., NSF | Regioselective Control of...
Authors: Carles Fuertes‐Espinosa; Alejandra Gómez‐Torres; Roser Morales‐Martínez; Antonio Rodríguez‐Fortea; Cristina García‐Simón; Felipe Gándara; Inhar Imaz; +5 Authors

doi: 10.1002/anie.201806140 , 10.1002/ange.201806140

pmid: 29917307

handle: 10261/199745

Purification of Uranium‐based Endohedral Metallofullerenes (EMFs) by Selective Supramolecular Encapsulation and Release

Abstract

AbstractSupramolecular nanocapsule 1⋅(BArF)8 is able to sequentially and selectively entrap recently discovered U2@C80 and unprecedented Sc2CU@C80, simply by soaking crystals of 1⋅(BArF)8 in a toluene solution of arc‐produced soot. These species, selectively and stepwise absorbed by 1⋅(BArF)8, are easily released, obtaining highly pure fractions of U2@C80 and Sc2CU@C80 in one step. Sc2CU@C80 represents the first example of a mixed metal actinide‐based endohedral metallofullerene (EMF). Remarkably, the host–guest studies revealed that 1⋅(BArF)8 is able to discriminate EMFs with the same carbon cage but with different encapsulated cluster and computational studies provide support for these observations.

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Keywords

Uranium, Supramolecular capsules, Endohedral metallofullerenes

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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
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