Physics-informed neural networks (PINNs) provide a new approach to solving partial differential equations (PDEs), while the properties of coupled physical laws present potential in surrogate modeling. However, the accuracy of PINNs in solving forward problems needs to be enhanced, and solving inverse problems relies on data samples. The smoothed finite element method (S-FEM) can obtain high-fidelity numerical solutions, which are easy to solve for the forward problems of PDEs, but difficult to solve for the inverse problems. To the best of the authors’ knowledge, there has been no prior research on coupling S-FEM and PINN. In this paper, a novel approach that couples S-FEM and PINN is proposed. The proposed approach utilizes S-FEM to synthesize high-fidelity datasets required for PINN inversion, while also improving the accuracy of data-independent PINN in solving forward problems. The proposed approach is applied to solve linear elastic and elastoplastic forward and inverse problems. The computational results demonstrate that the coupling of the S-FEM and PINN exhibits high precision and convergence when solving inverse problems, achieving a maximum relative error of 0.2% in linear elasticity and 5.69% in elastoplastic inversion by using approximately 10,000 data points. The coupling approach also enhances the accuracy of solving forward problems, reducing relative errors by approximately 2–10 times. The proposed coupling of the S-FEM and PINN offers a novel surrogate modeling approach that incorporates knowledge and data-driven techniques, enabling it to solve both forward and inverse problems associated with PDEs with high levels of accuracy and convergence.