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Effect of Concrete Waste Form Properties on Radionuclide Migration

Authors: Mattigod, Shas V.; Bovaird, Chase C.; Wellman, Dawn M.; Skinner, De'Chauna J.; Cordova, Elsa A.; Wood, Marcus I.;

Effect of Concrete Waste Form Properties on Radionuclide Migration

Abstract

The objective of this investigation was to initiate numerous sets of concrete-soil half-cell tests to quantify 1) diffusion of I and Tc from concrete into uncontaminated soil after 1 and 2 years, 2) I and Re (set 1) and Tc (set 2) diffusion from fractured concrete into uncontaminated soil, and 3) evaluate the moisture distribution profile within the sediment half-cell. These half-cells will be section in FY2009 and FY2010. Additionally, 1) concrete-soil half-cells initiated during FY2007 using fractured prepared with and without metallic iron, half of which were carbonated using carbonated, were sectioned to evaluate the diffusion of I and Re in the concrete part of the half-cell under unsaturated conditions (4%, 7%, and 15% by wt moisture content), 2) concrete-soil half cells containing Tc were sectioned to measure the diffusion profile in the soil half-cell unsaturated conditions (4%, 7%, and 15% by wt moisture content), and 3) solubility measurements of uranium solid phases were completed under concrete porewater conditions. The results of these tests are presented.

Country
United States
Related Organizations
Keywords

Aging, Iron, Waste Forms, 12 Management Of Radioactive Wastes, Precipitation, Distribution, Diffusion, Sediments, Ground Water, Radionuclide Migration, Concretes, Wastes, Moisture, Radioisotopes, And Non-Radioactive Wastes From Nuclear Facilities, Technetium, Rhenium, Retention, Solubility, Cements, Sorption, Soils, Uranium, Tanks, Iodine

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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
3
Average
Average
Average