Ultrasonic guided waves have been widely acknowledged as the most promising tools for nondestructive evaluation (NDE). However, because of the multimodal dispersion, the received guided modes usually overlap in both time and frequency, which highly complicates the mode separation and signal interpretation. The time-reversal technique can be used to realize the time recompression of the Lamb waves, but because of the multimode excitation and reception, it still may not be able to remove the mode ambiguity and achieve the pure pulse compression. With the goal of overcoming this limitation, a wideband dispersion reversal (WDR) technique is proposed. The technique makes use of a priori knowledge of the guided dispersion characteristics to synthesize the corresponding dispersion reversal excitations, which are able to selectively excite the self-compensation pure mode pulse. The theoretical basis of the technique is thoroughly described. A two-dimensional finite-difference time-domain (2D-FDTD) method is employed to simulate the propagation of two fundamental Lamb modes, the symmetrical S0 and antisymmetrical A0 modes in a steel plate. The proposed method was verified through experimental investigation. Finally, the advantages and potential applications of the method are briefly discussed.