Complete and precise characterization of a quantum dynamical process can be achieved via the method of quantum process tomography. Using a source of correlated photons, we have implemented several methods investigating a wide range of processes, e.g., unitary, decohering, and polarizing. One of these methods, ancilla-assisted process tomography (AAPT), makes use of an additional ``ancilla system,'' and we have theoretically determined the conditions when AAPT is possible. All prior schemes for AAPT make use of entangled states. Our results show that, surprisingly, entanglement is not required for AAPT, and we present process tomography data obtained using an input state that has no entanglement. However, the use of entanglement yields superior results.

To appear in Physical Review Letters