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Physical Review B
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Physical Review B
Article . 2008 . Peer-reviewed
License: APS Licenses for Journal Article Re-use
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Magnetic resonant x-ray diffraction study of europium telluride

Authors: B. Díaz; E. Granado; E. Abramof; P. H. O. Rappl; V. A. Chitta; A. B. Henriques;

Magnetic resonant x-ray diffraction study of europium telluride

Abstract

Here we use magnetic resonant x-ray diffraction to study the magnetic order in a $1.5\text{ }\ensuremath{\mu}\text{m}$ EuTe film grown on (111) ${\text{BaF}}_{2}$ by molecular-beam epitaxy. At $\text{Eu}\text{ }{L}_{\text{II}}$ and ${L}_{\text{III}}$ absorption edges, a resonant enhancement of more than two orders was observed for the $\ensuremath{\sigma}\ensuremath{\rightarrow}{\ensuremath{\pi}}^{\ensuremath{'}}$ diffracted intensity at half-order reciprocal-lattice points, consistent with the magnetic character of the scattering. We studied the evolution of the $(\frac{1}{2}\frac{1}{2}\frac{1}{2})$ magnetic reflection with temperature. When heating toward the Neel temperature $({T}_{N})$, the integrated intensity decreased monotonously and showed no hysteresis upon cooling again, indicating a second-order phase transition. A power-law fit to the magnetization versus temperature curve yielded ${T}_{N}=9.99(1)\text{ }\text{K}$ and a critical exponent $\ensuremath{\beta}=0.36(1)$, which agrees with the renormalization theory results for three-dimensional Heisenberg magnets. The fits to the sublattice magnetization dependence with temperature, disregarding and considering fourth-order exchange interactions, evidenced the importance of the latter for a correct description of magnetism in EuTe. A value of 0.009 was found for the $(2{j}_{1}+{j}_{2})/{J}_{2}$ ratio between the Heisenberg ${J}_{2}$ and fourth-order ${j}_{1,2}$ exchange constants. The magnetization curve exhibited a round-shaped region just near ${T}_{N}$ accompanied by an increase in the magnetic peak width, which was attributed to critical scattering above ${T}_{N}$. The comparison of the intensity ratio between the $(\frac{1}{2}\frac{1}{2}\frac{1}{2})$ and the $(1\frac{1}{2}1\frac{1}{2}1\frac{1}{2})$ magnetic reflections proved that the ${\text{Eu}}^{2+}$ spins align within the (111) planes, and the azimuthal dependence of the $(\frac{1}{2}\frac{1}{2}\frac{1}{2})$ magnetic peak is consistent with the model of equally populated S domains.

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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
17
Average
Top 10%
Top 10%
bronze