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Spatial Distribution of Nanocrystals Imaged at the Liquid-Air Interface

descriptionPublicationkeyboard_double_arrow_right Article 03 Sep 2013 Netherlands English Publisher:American Physical Society (APS)Journal:Physical Review Letters, volume 111 (issn: 0031-9007, eissn: 1079-7114,

Authors: Rijssel, J.; van der Linden, Marte; Meeldijk, J.D.; van Dijk-Moes, R.J.A.; Philipse, A.P.; Erné, B.H.;

doi: 10.1103/physrevlett.111.108302

pmid: 25166717

Spatial Distribution of Nanocrystals Imaged at the Liquid-Air Interface

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Abstract

The 3D distribution of nanocrystals at the liquid-air interface is imaged for the first time on a single-particle level by cryogenic electron tomography, revealing the equilibrium concentration profile from the interface to the bulk of the liquid. When the surface tension of the liquid is decreased, the interaction of the nanocrystals with the liquid-air interface shifts from adsorption to desorption. Macroscopic surface tension measurements do not detect this transition, due to the presence of surface-active molecular species.

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Netherlands

Related Organizations

Utrecht University
Netherlands

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