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Exciton lifetimes of CdTe nanocrystal quantum dots in high magnetic fields

Authors: Blokland, J.H.; Claessen, V.I.; Wijnen, F.J.P.; Groeneveld, E.; de Mello Donegá, C.; Vanmaekelbergh, D.A.M.; Meijerink, A.; +2 Authors

Exciton lifetimes of CdTe nanocrystal quantum dots in high magnetic fields

Abstract

We have measured the low-temperature (4.2 K) exciton lifetimes of zinc-blende CdTe nanocrystal quantum dots (NQDs), 2.6–3.8 nm in diameter, in magnetic fields up to 30 T. The exciton photoluminescence decay time decreases with both dot size and magnetic field. We explain the decrease in decay time in magnetic fields by the mixing of bright and dark exciton states due to a small shape asymmetry in the zinc-blende CdTe NQDs. We show that this behavior resembles that of wurtzite CdSe NQDs, and we demonstrate that an asymmetry of NQDs caused by either shape or crystal structure leads to similar exciton decay dynamics.

Country
Netherlands
Related Organizations
Keywords

Molecular and Biophysics, Correlated Electron Systems / High Field Magnet Laboratory (HFML)

  • BIP!
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    citations
    This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
    31
    popularity
    This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
    Top 10%
    influence
    This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
    Top 10%
    impulse
    This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
    Top 10%
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citations
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
31
Top 10%
Top 10%
Top 10%
Green
bronze