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https://doi.org/10.1103/physre...
Article . 2024 . Peer-reviewed
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https://dx.doi.org/10.48550/ar...
Article . 2023
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Topology of Bi2Se3 nanosheets

Authors: L. Maisel Licerán; S. J. H. Koerhuis; D. Vanmaekelbergh; H. T. C. Stoof;

Topology of Bi2Se3 nanosheets

Abstract

Recently, the quantum spin-Hall edge channels of two-dimensional colloidal nanocrystals of the topological insulator Bi$_2$Se$_3$ were observed directly. Motivated by this development, we reconsider the four-band effective model which has been traditionally employed in the past to describe thin nanosheets of this material. Derived from a three-dimensional $\boldsymbol{k} \boldsymbol{\cdot} \boldsymbol{p}$ model, it physically describes the top and bottom electronic surface states at the $Γ$ point that become gapped due to the material's small thickness. However, we find that the four-band model for the surface states alone, as derived directly from the three-dimensional theory, is inadequate for the description of thin films of a few quintuple layers and even yields an incorrect topological invariant within a significant range of thicknesses. To address this limitation we propose an eight-band model which, in addition to the surface states, also incorporates the set of bulk states closest to the Fermi level. We find that the eight-band model not only captures most of the experimental observations, but also agrees with previous first-principles calculations of the $\mathbb{Z}_{2}$ invariant in thin films of varying thickness. The band inversion around the $Γ$ point, which endows the surface-like bands with topology, is shown to be enabled by the presence of the additional bulk-like states without requiring any reparametrization of the resulting effective Hamiltonian.

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Netherlands
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Keywords

Condensed Matter - Other Condensed Matter, Condensed Matter - Materials Science, Quantum Physics, Condensed Matter - Mesoscale and Nanoscale Physics, Mesoscale and Nanoscale Physics (cond-mat.mes-hall), Materials Science (cond-mat.mtrl-sci), FOS: Physical sciences, Condensed Matter Physics, Quantum Physics (quant-ph), Electronic, Optical and Magnetic Materials, Other Condensed Matter (cond-mat.other)

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citations
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
1
Average
Average
Average
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