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Journal of Physics Condensed Matter
Article . 2012 . Peer-reviewed
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Transient dynamics in dense colloidal suspensions under shear: shear rate dependence

Authors: Laurati M.; Mutch K. J.; Koumakis N.; Zausch J.; Amann C. P.; Schofield A. B.; Petekidis G.; +4 Authors

Transient dynamics in dense colloidal suspensions under shear: shear rate dependence

Abstract

A combination of confocal microscopy and rheology experiments, Brownian dynamics (BD) and molecular dynamics (MD) simulations and mode coupling theory (MCT) have been applied in order to investigate the effect of shear rate on the transient dynamics and stress-strain relations in supercooled and glassy systems under shear. Immediately after shear is switched on, the microscopic dynamics display super-diffusion and the macroscopic rheology a stress overshoot, which become more pronounced with increasing shear rate. MCT relates both to negative sections of the generalized shear modulus, which grow with increasing shear rate. When the inverse shear rate becomes much smaller than the structural relaxation time of the quiescent system, relaxation through Brownian motion becomes less important. In this regime, larger stresses are accumulated before the system yields and the transition from localization to flow occurs earlier and more abruptly.

Countries
Germany, United States, Italy
Keywords

Colloids, Dynamics, Glasses, Confocal Microscopy, Shear, mechanical & thermal, Chemical physics and physical chemistry, info:eu-repo/classification/pacs/82.70.Dd Colloids; 62.10.+s Mechanical properties of liquids; 82.70.Kj Emulsions and suspensions; 61.20.Ja Computer simulation of liquid structure; 64.70.P- Glass transitions of specific systems, liquids and polymers, Soft matter, Condensed matter: structural, info:eu-repo/classification/ddc/530, 530

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citations
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
47
Top 10%
Top 10%
Top 10%
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bronze
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