To determine the relative contributions of galactic and intracluster stars to the enrichment of the intracluster medium (ICM), we present X-ray surface brightness, temperature, and Fe abundance profiles for a set of twelve galaxy clusters for which we have extensive optical photometry. Assuming a standard IMF and simple chemical evolution model scaled to match the present-day cluster early-type SN Ia rate, the stars in the brightest cluster galaxy (BCG) plus the intracluster stars (ICS) generate 31^{+11}_{-9}%, on average, of the observed ICM Fe within r_{500} (~ 0.6 times r_{200}, the virial radius). An alternate, two-component SN Ia model (including both prompt and delayed detonations) produces a similar BCG+ICS contribution of 22^{+9}_{-9}%. Because the ICS typically contribute 80% of the BCG+ICS Fe, we conclude that the ICS are significant, yet often neglected, contributors to the ICM Fe within r_{500}. However, the BCG+ICS fall short of producing all the Fe, so metal loss from stars in other cluster galaxies must also contribute. By combining the enrichment from intracluster and galactic stars, we can account for all the observed Fe. These models require a galactic metal loss fraction (0.84^{+0.11}_{-0.14}) that, while large, is consistent with the metal mass not retained by galactic stars. The SN Ia rates, especially as a function of galaxy environment and redshift, remain a significant source of uncertainty in further constraining the metal loss fraction. For example, increasing the SN Ia rate by a factor of 1.8 -- to just within the 2 sigma uncertainty for present-day cluster early-type galaxies -- allows the combined BCG + ICS + cluster galaxy model to generate all the ICM Fe with a much lower galactic metal loss fraction (~ 0.35).

27 pages, 9 figures, 7 tables. Accepted for publication in ApJ