Small molecules that interact strongly with water were the subject of this molecular dynamics (MD) study. These solutes include a cryoprotectant (DMSO), a polyalcohol [CH2(OH)2], carboxylic acid conjugates (HCOOH and HCOONa), an ammonium salt (NH4Cl), and two alkyl halide salts (NaCl and NaF). MD simulations were carried out for bulk supercooled liquids and solutions in contact with ice. Solute and water hydrogen bonding, orientational and translational order, and hydrogen bond jump dynamics were compared in bulk and as a function of distance from the solute molecules. Reverse non-equilibrium molecular dynamics simulations were used to determine interfacial widths, friction coefficients (κ) with ice, and solution phase viscosities (η). Ionic solutes were found to reduce orientational and translational ordering near the ice interfaces. However, in bulk liquids, we find a correlation between orientational ordering and the statistics of water hydrogen bonds—a donor–acceptor imbalance in water has the greatest impact on ordering in the bulk liquids. Although ionic solutions exhibited similar effects on the water structure, the effect on dynamics depends most directly on donor–acceptor imbalance. Solutes that are hydrogen bond acceptors were found to slow hydrogen bond lifetimes relative to hydrogen bond donors. We also observed a direct correlation between the liquid phase hydrogen-bond jump times and shear viscosity. Finally, of all the solutes studied, only DMSO and sodium formate exhibited increased friction at the ice–water interface.