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Applied Physics Letters
Article . 2023 . Peer-reviewed
Data sources: Crossref
https://dx.doi.org/10.48550/ar...
Article . 2023
License: CC BY
Data sources: Datacite
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Improper ferroelectricity in ultrathin hexagonal ferrites films

Authors: Xin Li; Yu Yun; Xiaoshan Xu;

Improper ferroelectricity in ultrathin hexagonal ferrites films

Abstract

Suppression of ferroelectricity in ultrathin films of improper ferroelectric hexagonal ferrites or manganites has been attributed to the effect of interfacial clamping; however, the quantitative understanding and related phenomenological model are still lacking. In this work, we report on the paraelectric-to-ferroelectric phase transition of epitaxial h-ScFeO3 films with different thicknesses through in situ reflection high-energy electron diffraction. Based on the interfacial clamping model and the Landau theory, we show that the thickness-dependence of the ferroelectric Curie temperature can be understood in terms of the characteristic length of an interfacial clamping layer and the bulk Curie temperature. Furthermore, we found that the critical thickness of improper ferroelectricity is proportional to the characteristic length of the interfacial clamping layer. These results reveal the essential role of mechanical clamping from interface on the improper ferroelectricity of hexagonal ferrites or manganites and could serve as the guidance to achieve robust improper ferroelectricity in ultrathin films.

Country
United States
Keywords

Physics, Materials Science, Physical Sciences and Mathematics, 500, Materials Science (cond-mat.mtrl-sci), FOS: Physical sciences, 530

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    influence
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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
4
Top 10%
Average
Average
Green