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pmid: 27822486
pmc: PMC5074990
We review our recent time- and angle-resolved photoemission spectroscopy experiments, which measure the transient electronic structure of optically driven graphene. For pump photon energies in the near infrared (ℏωpump=950 meV), we have discovered the formation of a population-inverted state near the Dirac point, which may be of interest for the design of THz lasing devices and optical amplifiers. At lower pump photon energies (ℏωpump<400 meV), for which interband absorption is not possible in doped samples, we find evidence for free carrier absorption. In addition, when mid-infrared pulses are made resonant with an infrared-active in-plane phonon of bilayer graphene (ℏωpump=200 meV), a transient enhancement of the electron-phonon coupling constant is observed, providing interesting perspective for experiments that report light-enhanced superconductivity in doped fullerites in which a similar lattice mode was excited. All the studies reviewed here have important implications for applications of graphene in optoelectronic devices and for the dynamical engineering of electronic properties with light.
Condensed Matter - Materials Science, Crystallography, Condensed Matter - Mesoscale and Nanoscale Physics, QD901-999, Mesoscale and Nanoscale Physics (cond-mat.mes-hall), Topical Reviews, Materials Science (cond-mat.mtrl-sci), FOS: Physical sciences
Condensed Matter - Materials Science, Crystallography, Condensed Matter - Mesoscale and Nanoscale Physics, QD901-999, Mesoscale and Nanoscale Physics (cond-mat.mes-hall), Topical Reviews, Materials Science (cond-mat.mtrl-sci), FOS: Physical sciences
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