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Nucleophilicity scale for n- and π-nucleophiles

descriptionPublicationkeyboard_double_arrow_right Article 01 Aug 2006 Chile English Publisher:Elsevier BVJournal:Chemical Physics Letters, volume 427, pages 421-425 (issn: 0009-2614, Copyright policy )
Authors: Jaramillo, Paula; Fuentealba Rosas, Patricio; Pérez, Patricia;

doi: 10.1016/j.cplett.2006.06.066

handle: 10533/177780 , 10533/177779

Nucleophilicity scale for n- and π-nucleophiles

Abstract

Abstract A recently introduced empirical nucleophilicity index for a series of n- and π-nucleophiles was evaluated. The index is based on the frontier molecular orbital information of the nucleophile and its electrophilic partner. The model is validated against kinetic data of alkenes, phosphanes, phosphites and amines interacting with the corresponding electrophilic partner. The predictive character of this index is tested for some nucleophiles.

Country
Chile
Related Organizations
Keywords

Physics and Astronomy (all), DIELS-ALDER REACTIONS, Physical and Theoretical Chemistry

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    This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
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    popularity
    This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
    		 Top 10%
    influence
    This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
    		 Top 10%
    impulse
    This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
    		 Top 10%
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selected citations
These citations are derived from selected sources.
This is an alternative to the "Influence" indicator, which also reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Citations provided by BIP!
popularity
This indicator reflects the "current" impact/attention (the "hype") of an article in the research community at large, based on the underlying citation network.
BIP!Popularity provided by BIP!
influence
This indicator reflects the overall/total impact of an article in the research community at large, based on the underlying citation network (diachronically).
BIP!Influence provided by BIP!
impulse
This indicator reflects the initial momentum of an article directly after its publication, based on the underlying citation network.
BIP!Impulse provided by BIP!
34
Top 10%
Top 10%
Top 10%
Green