In an effort to extend the available manufacturing technologies for Ti3Albase aluminides, the potential success of a new hot-rolling process for the production of high-quality foils has been investigated. Processing of Super-α2 aluminide foils approximately 0.15 mm thick takes full advantage of the combined benefits of controlled rolling and a unique pack rolling process. Based on the results of a study of phase transformation kinetics, microstructure and hardness of continuously-cooled and isothermally transformed specimens, the processing parameters are optimized to provide enhanced surface quality and superior ductilities in the as-rolled condition.