Helicity is an important physical variable which is similar to the energy and enstrophy in three-dimensional fluid. It can be used to describe the motion in the direction of fluid rotation and also can be regarded as a new physical variable in turbulence theory. In recent years, it has been used in atmospheric dynamics. In this paper, helicity of atmospheric flow, especially helicity in the boundary layer and in the vicinity of front was discussed. These results show that helicity is usually positive in the boundary layer due to the effect of friction. The helicity of boundary layer flow is larger in anticyclone than that in cyclone, resulting from the different wind structures of boundary layers in anticyclone and cyclone under the geostrophic momentum approximation. It is possible that the helicity is negative at certain height in the baroclinic boundary layer. The influences of nonlinearity and baroclinity on the helicity are important. The so called “Cloud Street” in the boundary layer is related to the dynamics of helicity. Helicity in the atmosphere can be expressed as the temperature advection under some conditions, so helicity would be allowed to describe the frontogenesis and development of frontal structure. The amplitude of helicity increases with time in the frontogenesis. A large gradient of helicity is generated in the region located to the northeast of the surface low and in which the front is formed. In warm frontal region, as well as behind the trough of temperature, the helicity is positive, while the helicity is negative in cold frontal sector and in the ahead ridge of temperature. The largest helicity occurs in the boundary.